{
  "abstract": "Electrostatic complex coacervates offer a robust pathway to convert homogeneous oppositely charged polyelectrolyte solutions into condensed structured liquids via liquid–liquid phase separation (LLPS). Directing these principles toward artificial, all‐proteinaceous complex coacervates enables the development of soft matter systems fully compatible with a broad range of advanced biotechnological products. Here, we employ charge‐tunable β‐lactoglobulin and lysozyme amyloid nanofibrils as building blocks toward fully proteinaceous functional materials. The functionality is dictated by engineering the composition and self‐organization of oppositely charged amyloid nanofibrils at the liquid–liquid interface. Depending on the path and process followed, we demonstrate all‐amyloid interfacial complex coacervates in the form of vein‐like tubular structures or capsules with tunable electrical or ionic conductivity, viscoelasticity, multidimensional morphology, and programmable macromolecular crowding. These constructs, made solely of amyloid constituents, provide a general platform for artificial protein scaffolds and advanced materials with potential applications in bioelectronics and bio‐optics.",
  "abstract_shown": true,
  "affiliations": [
    "Nanomaterials and Polymer Nanocomposites Laboratory School of Engineering University of British Columbia Kelowna BC Canada",
    "Department of Health Sciences and Technology ETH Zürich Zürich Switzerland",
    "Department of Materials ETH Zürich Zürich Switzerland"
  ],
  "article_type": "research article",
  "arxiv": null,
  "author_total": 5,
  "authors": [
    {
      "affs": [
        0,
        1
      ],
      "name": "Seyyed Alireza Hashemi",
      "orcid": "0000-0002-4713-6883"
    },
    {
      "affs": [
        1
      ],
      "name": "Mohammad Peydayesh",
      "orcid": "0000-0002-6265-3811"
    },
    {
      "affs": [
        1
      ],
      "name": "Laura Baraldi"
    },
    {
      "affs": [
        0
      ],
      "name": "Mohammad Arjmand"
    },
    {
      "affs": [
        1,
        2
      ],
      "name": "Raffaele Mezzenga",
      "orcid": "0000-0002-5739-2610"
    }
  ],
  "bibtex": "https://research.draconitic.com/paper/7xa8nqj76watn.bib",
  "cited_by": 0,
  "doi": "10.1002/adma.74737",
  "fulltext_url": "https://pmc.ncbi.nlm.nih.gov/articles/PMC13726710/",
  "id": "7xa8nqj76watn",
  "issns": [
    "0935-9648",
    "1521-4095"
  ],
  "landing_url": "https://doi.org/10.1002/adma.74737",
  "language": "en",
  "licence": "CC-BY-4.0",
  "licence_label": "CC BY 4.0",
  "licence_source": "article",
  "licence_url": "https://creativecommons.org/licenses/by/4.0/",
  "metadata_licence": null,
  "native_subjects": [
    [
      "heading",
      "Research Article"
    ],
    [
      "openalex",
      "2502|Supramolecular Self-Assembly in Materials"
    ]
  ],
  "openalex": "W7204097412",
  "pdf_url": null,
  "pmcid": "PMC13726710",
  "pmid": "42635593",
  "published": "2026-08-24",
  "publisher": null,
  "ris": "https://research.draconitic.com/paper/7xa8nqj76watn.ris",
  "sources": [
    {
      "first_seen": "2026-11-05T12:22:59Z",
      "native_id": "PMC13726710",
      "source": "pmc",
      "url": "https://doi.org/10.1002/adma.74737"
    }
  ],
  "subjects": [
    {
      "field": "chemistry",
      "origin": "openalex:2502|Supramolecular Self-Assembly in Materials",
      "subfield": "materials-polymers"
    }
  ],
  "title": "All‐Amyloid Functional Coacervates",
  "title_text": "All‐Amyloid Functional Coacervates",
  "type": "peer-reviewed",
  "updated_at": "2026-11-06T12:22:35Z",
  "url": "https://research.draconitic.com/paper/7xa8nqj76watn",
  "venue": "Advanced Materials (Deerfield Beach, Fla.)",
  "versions": []
}