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PreprintCC BY 4.0arXiv

Staged emergence of anomalous Hall transport in a correlated uranium Weyl semimetal

Abstract

Understanding how electronic correlations reshape topological states remains a central challenge in quantum materials. Here we investigate the uranium ferromagnet UPS using magnetotransport, angle-resolved photoemission spectroscopy, thermodynamic measurements, and first principles calculations. Resonant photoemission reveals narrow U-5f spectral weight at the Fermi level coexisting with broad incoherent states, consistent with the itinerant/localized duality characteristic of uranium 5f electrons. The anomalous Hall conductivity reaches approximately 4.5×102 Ω−1cm−1, yet does not simply follow the ordered magnetic moment. Temperature dependent photoemission reveals relatively little change across TC=118~K, followed by a pronounced redistribution of low-energy 5f spectral weight below approximately 90~K. First-principles calculations identify a symmetry protected Weyl crossing with pronounced Berry curvature and yield an intrinsic anomalous Hall conductivity of approximately 9.6×102 Ω−1cm−1. These results demonstrate that magnetic order, correlated electronic reconstruction, and anomalous Hall transport develop over distinct but overlapping temperature ranges, revealing how strong correlations reshape topological transport in a uranium Weyl semimetal.

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BibTeX
@misc{regmi2026staged,
  title = {{Staged emergence of anomalous Hall transport in a correlated uranium Weyl semimetal}},
  author = {Sabin Regmi and Shuxiang Zhou and Chandan K. Singh and Alexei Fedorov and Jonathan Denlinger and Zeyu Ma and Yidi Wang and Jennifer E. Hoffman and Peter M. Oppeneer and Dariusz Kaczorowski and Tomasz Durakiewicz and Krzysztof Gofryk},
  howpublished = {arXiv},
  year = {2026},
  month = sep,
  doi = {10.48550/arxiv.2609.24897},
  eprint = {2609.24897},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2609.24897},
  note = {CC BY 4.0},
}
RIS
TY  - UNPB
TI  - Staged emergence of anomalous Hall transport in a correlated uranium Weyl semimetal
AU  - Sabin Regmi
AU  - Shuxiang Zhou
AU  - Chandan K. Singh
AU  - Alexei Fedorov
AU  - Jonathan Denlinger
AU  - Zeyu Ma
AU  - Yidi Wang
AU  - Jennifer E. Hoffman
AU  - Peter M. Oppeneer
AU  - Dariusz Kaczorowski
AU  - Tomasz Durakiewicz
AU  - Krzysztof Gofryk
PY  - 2026
DA  - 2026/09/21
PB  - arXiv
DO  - 10.48550/arxiv.2609.24897
UR  - https://arxiv.org/abs/2609.24897
AB  - Understanding how electronic correlations reshape topological states remains a central challenge in quantum materials. Here we investigate the uranium ferromagnet UPS using magnetotransport, angle-resolved photoemission spectroscopy, thermodynamic measurements, and first principles calculations. Resonant photoemission reveals narrow U-5f spectral weight at the Fermi level coexisting with broad incoherent states, consistent with the itinerant/localized duality characteristic of uranium 5f electrons. The anomalous Hall conductivity reaches approximately 4.5×10^2 Ω^−1cm^−1, yet does not simply follow the ordered magnetic moment. Temperature dependent photoemission reveals relatively little change across T_C=118~K, followed by a pronounced redistribution of low-energy 5f spectral weight below approximately 90~K. First-principles calculations identify a symmetry protected Weyl crossing with pronounced Berry curvature and yield an intrinsic anomalous Hall conductivity of approximately 9.6×10^2 Ω^−1cm^−1. These results demonstrate that magnetic order, correlated electronic reconstruction, and anomalous Hall transport develop over distinct but overlapping temperature ranges, revealing how strong correlations reshape topological transport in a uranium Weyl semimetal.
ER  -