Skip to content
DraconiticResearch
Search Sources API
186,541 studies31 sourcesUpdated 53 min ago
PreprintCC BYChemRxiv

P,T-odd sensitivity parameters of laser-coolable SrOH from relativisticcoupled-cluster theory

  • Kaushik Talukdar1,2
  • Himangshu Das1,2
  • Sishmita Tamang1,2
  • Malaya K Nayak3,4,5
5 affiliations
  1. 1Department of Chemical and Biological Sciences
  2. 2National Institute of Technology Meghalaya
  3. 3Theoretical Chemistry Section
  4. 4Bhabha Atomic Research Centre
  5. 5BARC Training School Complex
Open at sourcePDFDOICite

Abstract

Ultracold molecules have attracted significant interest as promising platforms for exploring fundamental physics and quantum information science. As progress toward precision measurements with the ultracold SrOH molecule is currently underway [{\it Phys. Rev. Lett. 134, 083401 (2025)}], we present a four-component relativistic coupled-cluster (RCC) study of various parity- and time-reversal-violating (P,T-odd) interactions in the ground electronic state of SrOH. In particular, we extend the application of the Z-vector (energy-derivative) approach within the RCC framework to a polyatomic molecule for the calculation of P,T-odd molecular sensitivity parameters. We obtain the following molecular parameters for SrOH: Eeff = 2.12 ± 0.27~GV/cm, WS = 1.89 ± 0.21~kHz, and WM = (2.04 ± 0.12) × 1032~Hz/e·cm2. These parameters provide essential molecular inputs for the design and interpretation of precision experiments with SrOH. We find that the P,T-odd sensitivity parameters of SrOH are comparable to those of the isoelectronic diatomic molecule SrF. However, the polyatomic structure of SrOH offers enhanced capabilities for suppressing systematic errors, making it a particularly promising candidate for high-precision searches for P,T violation.

Related

  1. Sensitivity of kinematics to biomechanical model parameters in markerless motion analysis
    Antoine Muller, Martin Dizier, Mathis Renaudin +1
    Multidisciplinary Biomechanics JournalPeer-reviewedCC BY 4.0Full textGeneral physicsHAL
  2. A Hybrid Simulation Code for Hall Thrusters and its Sensitivity to Numerical Parameters
    Xingdong Che, Hong Li, Xin Guo +3
    arXivPreprintarXiv licenceFull textPlasma physicsarXiv
  3. Non-stick vacuum wall collisions with a laser-coolable molecule
    P. Kukreja, L. A. Rautenberg, J. C. Blumenstock +3
    arXivPreprintCC BY 4.0Full textAtomic, molecular & optical physicsarXiv
  4. Sensitivity analysis of annual energy production and associated economic losses due to external wake effects on offshore wind clusters: A case study of the Shinan offshore wind cluster in southwest sea of Korea
    Geonhwa Ryu, Dohee Lee, Jungho Kim +4
    PLOS OnePeer-reviewedCC BY 4.0Full textAtmospheric science & meteorologyFluid dynamicsPLOS
  5. Fock-space relativistic coupled-cluster study of systematic shifts and fine-structure constant sensitivity in {\rm Cf17+}, {\rm Cm15+} and {\rm Bk16+} highly charged ions
    Palki Gakkhar, D. Angom, B. K. Mani
    arXivPreprintCC BY 4.0Full textAtomic, molecular & optical physicsarXiv

Cite

BibTeXRIS
BibTeX
@misc{talukdar2026ptodd,
  title = {{P,T-odd sensitivity parameters of laser-coolable SrOH from relativisticcoupled-cluster theory}},
  author = {Kaushik Talukdar and Himangshu Das and Sishmita Tamang and Malaya K Nayak},
  howpublished = {ChemRxiv},
  year = {2026},
  month = sep,
  doi = {10.26434/chemrxiv.10001729/v2},
  url = {https://chemrxiv.org/doi/full/10.26434/chemrxiv.10001729/v2},
  note = {CC BY},
}
RIS
TY  - UNPB
TI  - P,T-odd sensitivity parameters of laser-coolable SrOH from relativisticcoupled-cluster theory
AU  - Kaushik Talukdar
AU  - Himangshu Das
AU  - Sishmita Tamang
AU  - Malaya K Nayak
PY  - 2026
DA  - 2026/09/14
PB  - ChemRxiv
DO  - 10.26434/chemrxiv.10001729/v2
UR  - https://chemrxiv.org/doi/full/10.26434/chemrxiv.10001729/v2
AB  - Ultracold molecules have attracted significant interest as promising platforms for exploring fundamental physics and quantum information science. As progress toward precision measurements with the ultracold SrOH molecule is currently underway [{\it Phys. Rev. Lett. 134, 083401 (2025)}], we present a four-component relativistic coupled-cluster (RCC) study of various parity- and time-reversal-violating (P,T-odd) interactions in the ground electronic state of SrOH. In particular, we extend the application of the Z-vector (energy-derivative) approach within the RCC framework to a polyatomic molecule for the calculation of P,T-odd molecular sensitivity parameters. We obtain the following molecular parameters for SrOH: E_eff = 2.12 ± 0.27~GV/cm, W_S = 1.89 ± 0.21~kHz, and W_M = (2.04 ± 0.12) × 10^32~Hz/e·cm^2. These parameters provide essential molecular inputs for the design and interpretation of precision experiments with SrOH. We find that the P,T-odd sensitivity parameters of SrOH are comparable to those of the isoelectronic diatomic molecule SrF. However, the polyatomic structure of SrOH offers enhanced capabilities for suppressing systematic errors, making it a particularly promising candidate for high-precision searches for P,T violation.
ER  -