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PreprintarXiv licencearXiv

Floquet-Volkov spin polarization in spin-degenerate Antiferromagnets

Abstract

Periodic driving enables ultrafast control of electronic structures in solids through the formation of photon-dressed Floquet-Bloch states. However, the measured photoemission spectra are influenced not only by these states but also by their interference with Volkov-dressed outgoing photoelectrons. Here, we demonstrate that Floquet-Volkov interference can generate spin-polarized photoemission in a collinear antiferromagnetic Dirac model without spin-orbit coupling (SOC). An in-plane linearly polarized pump preserves 𝒫𝒯 symmetry, leaving the Floquet quasienergies spin degenerate. Under near-resonant driving, photon-dressed conduction and valence bands hybridize, producing spin-dependent relative phases that are converted into unequal spin-resolved photoemission intensities through interference between pathways reaching the same Volkov-dressed final state. We analytically identify this interference mechanism and verify it using nonequilibrium Green-function calculations under periodic driving and finite pump-probe pulses. We further demonstrate that rotating the probe polarization can suppress or reverse the spin polarization without modifying the Floquet bands. Our findings establish Floquet-Volkov interference as a route to spin-selective photoemission in driven antiferromagnets without Floquet spin splitting or SOC.

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BibTeX
@misc{fan2026floquetvolkov,
  title = {{Floquet-Volkov spin polarization in spin-degenerate Antiferromagnets}},
  author = {Jiyang Fan and Dinghui Wang and Tongshuai Zhu},
  howpublished = {arXiv},
  year = {2026},
  month = nov,
  doi = {10.48550/arxiv.2611.05856},
  eprint = {2611.05856},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2611.05856},
}
RIS
TY  - UNPB
TI  - Floquet-Volkov spin polarization in spin-degenerate Antiferromagnets
AU  - Jiyang Fan
AU  - Dinghui Wang
AU  - Tongshuai Zhu
PY  - 2026
DA  - 2026/11/04
PB  - arXiv
DO  - 10.48550/arxiv.2611.05856
UR  - https://arxiv.org/abs/2611.05856
AB  - Periodic driving enables ultrafast control of electronic structures in solids through the formation of photon-dressed Floquet-Bloch states. However, the measured photoemission spectra are influenced not only by these states but also by their interference with Volkov-dressed outgoing photoelectrons. Here, we demonstrate that Floquet-Volkov interference can generate spin-polarized photoemission in a collinear antiferromagnetic Dirac model without spin-orbit coupling (SOC). An in-plane linearly polarized pump preserves 𝒫𝒯 symmetry, leaving the Floquet quasienergies spin degenerate. Under near-resonant driving, photon-dressed conduction and valence bands hybridize, producing spin-dependent relative phases that are converted into unequal spin-resolved photoemission intensities through interference between pathways reaching the same Volkov-dressed final state. We analytically identify this interference mechanism and verify it using nonequilibrium Green-function calculations under periodic driving and finite pump-probe pulses. We further demonstrate that rotating the probe polarization can suppress or reverse the spin polarization without modifying the Floquet bands. Our findings establish Floquet-Volkov interference as a route to spin-selective photoemission in driven antiferromagnets without Floquet spin splitting or SOC.
ER  -