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PreprintCC BY 4.0arXiv

Multiorbital periodic Anderson model for CeRh2As2

Abstract

CeRh2As2 is a heavy-fermion superconductor that exhibits distinct low- and high-field superconducting phases, widely interpreted as reflecting a field-induced change in the parity of the order parameter. However, the superconductivity develops in close proximity to magnetic order whose microscopic origin and nature remain unclear. Moreover, the low-lying crystal-electric-field-split doublets of the Ce 4f electrons appear to realize an unusual "quasi-quartet" structure. This has motivated proposals that quadrupolar degrees of freedom play an important role in the low-temperature physics. Here we develop a microscopic heavy-fermion description of CeRh2As2 that incorporates both the quasi-quartet structure and the nonsymmorphic symmetry. Within a multiorbital periodic Anderson model, we include the lowest-lying Γ7 and Γ6 doublets of the Ce 4f electrons, and allow for nonlocal hybridization with the conduction d electrons. Single occupancy of the 4f states is enforced within the rotationally invariant slave-boson formalism. Adopting a mean-field treatment, we first show that the effective low-energy Hamiltonian is accurately captured by a single-orbital tight-binding model, justifying the minimal descriptions widely employed in the literature. Allowing for a magnetic ground state, we find that our model displays metallic Q=(π,π) antiferromagnetic order over a wide parameter regime. Ferromagnetic solutions also occur, but in a smaller region of parameter space and with greater sensitivity to carrier concentration and the form of the f-d hybridization. Quadrupolar moments appear only within magnetically ordered phases and are generally small, becoming substantial only when the Γ7 and Γ6 doublets are nearly degenerate. Our results provide a microscopic basis for understanding the itinerant heavy-fermion physics and ordered phases of CeRh2As2.

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BibTeX
@misc{hackner2026multiorbital,
  title = {{Multiorbital periodic Anderson model for CeRh2As2}},
  author = {Nico A. Hackner and Changhee Lee and P. M. R. Brydon},
  howpublished = {arXiv},
  year = {2026},
  month = sep,
  doi = {10.48550/arxiv.2609.31001},
  eprint = {2609.31001},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2609.31001},
  note = {CC BY 4.0},
}
RIS
TY  - UNPB
TI  - Multiorbital periodic Anderson model for CeRh2As2
AU  - Nico A. Hackner
AU  - Changhee Lee
AU  - P. M. R. Brydon
PY  - 2026
DA  - 2026/09/25
PB  - arXiv
DO  - 10.48550/arxiv.2609.31001
UR  - https://arxiv.org/abs/2609.31001
AB  - CeRh2As2 is a heavy-fermion superconductor that exhibits distinct low- and high-field superconducting phases, widely interpreted as reflecting a field-induced change in the parity of the order parameter. However, the superconductivity develops in close proximity to magnetic order whose microscopic origin and nature remain unclear. Moreover, the low-lying crystal-electric-field-split doublets of the Ce 4f electrons appear to realize an unusual "quasi-quartet" structure. This has motivated proposals that quadrupolar degrees of freedom play an important role in the low-temperature physics. Here we develop a microscopic heavy-fermion description of CeRh2As2 that incorporates both the quasi-quartet structure and the nonsymmorphic symmetry. Within a multiorbital periodic Anderson model, we include the lowest-lying Γ_7 and Γ_6 doublets of the Ce 4f electrons, and allow for nonlocal hybridization with the conduction d electrons. Single occupancy of the 4f states is enforced within the rotationally invariant slave-boson formalism. Adopting a mean-field treatment, we first show that the effective low-energy Hamiltonian is accurately captured by a single-orbital tight-binding model, justifying the minimal descriptions widely employed in the literature. Allowing for a magnetic ground state, we find that our model displays metallic Q=(π,π) antiferromagnetic order over a wide parameter regime. Ferromagnetic solutions also occur, but in a smaller region of parameter space and with greater sensitivity to carrier concentration and the form of the f-d hybridization. Quadrupolar moments appear only within magnetically ordered phases and are generally small, becoming substantial only when the Γ_7 and Γ_6 doublets are nearly degenerate. Our results provide a microscopic basis for understanding the itinerant heavy-fermion physics and ordered phases of CeRh2As2.
ER  -