Electrical Spectroscopy of Intervalley Relaxation in WSe2 Transistors
Abstract
We show that the transconductance of multilayer WSe2 field-effect transistors serves as a direct electrical spectrometer of the intervalley relaxation time τiv, previously accessible only by ultrafast optical techniques. Extending an equilibrium valley-thermodynamics framework with a single relaxation equation for the Γ-valley carrier fraction fΓ(t), we predict three signatures: (i)~a Lorentzian transconductance gm(ω)=gm,0+gm,v0/(1+iωτiv), whose imaginary part peaks at ωc=τiv−1 with opposite signs for bilayer and trilayer; (ii)~a two-stage current transient after a gate step, exhibiting bilayer overshoot or trilayer undershoot; and (iii)~sweep-rate-proportional hysteresis whose gate-voltage profile and the layer-dependent transconductance sign reversal distinguish valley from trap-induced dynamics. All three signatures provide quantitative electrical access to τiv with standard radio-frequency (rf) and direct-current (dc) instrumentation.
Versions
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BibTeX
@misc{wakabayashi2026electrical,
title = {{Electrical Spectroscopy of Intervalley Relaxation in WSe$_2$ Transistors}},
author = {Katsunori Wakabayashi},
howpublished = {arXiv},
year = {2026},
month = jul,
doi = {10.48550/arxiv.2606.10470},
eprint = {2606.10470},
archivePrefix = {arXiv},
url = {https://arxiv.org/abs/2606.10470},
note = {CC BY 4.0},
}
RIS
TY - UNPB
TI - Electrical Spectroscopy of Intervalley Relaxation in WSe_2 Transistors
AU - Katsunori Wakabayashi
PY - 2026
DA - 2026/07/13
PB - arXiv
DO - 10.48550/arxiv.2606.10470
UR - https://arxiv.org/abs/2606.10470
AB - We show that the transconductance of multilayer WSe_2 field-effect transistors serves as a direct electrical spectrometer of the intervalley relaxation time τ_iv, previously accessible only by ultrafast optical techniques. Extending an equilibrium valley-thermodynamics framework with a single relaxation equation for the Γ-valley carrier fraction f_Γ(t), we predict three signatures: (i)~a Lorentzian transconductance g_m(ω)=g_m,0+g_m,v^0/(1+iωτ_iv), whose imaginary part peaks at ω_c=τ_iv^−1 with opposite signs for bilayer and trilayer; (ii)~a two-stage current transient after a gate step, exhibiting bilayer overshoot or trilayer undershoot; and (iii)~sweep-rate-proportional hysteresis whose gate-voltage profile and the layer-dependent transconductance sign reversal distinguish valley from trap-induced dynamics. All three signatures provide quantitative electrical access to τ_iv with standard radio-frequency (rf) and direct-current (dc) instrumentation.
ER -