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Peer-reviewedCC BY-NC-ND 4.0Communications Physics

Accessing the fundamental link between atomic populations and frequency distribution of spectral lines of ions in dense plasmas

6 more authors

Abstract

Dense plasmas enable to test our fundamental understanding of matter but a lack of data hindered searches of new physics in the past. A game changer is the new and unique Stanford-Linear-Accelerator-Center allowing X-ray line-shape-resolved resonance pumping via a combination of the self-seeded Linac-Coherent-Light-Source beam with an optical-laser produced dense plasma: Non-isolated atom models can now be benchmarked via the spectral distribution. High-precision spectroscopy reveals significant and simultaneous redistribution in population and frequency for transitions in He-like Vanadium. A critical principal quantum number is identified above which a strong intensity enhancement of higher lying Rydberg-lines appears although the corresponding ionic levels are not directly pumped. The Rydberg-lines themselves show significant distortions of their spectral distribution. We determine their frequency distributions with a precision of 0.2eV at 6.6keV and observe significant systematic deviations from available numerical methods. Our data question the current understanding how local thermodynamic equilibrium can be achieved. They also serve as a crucial benchmark for quantum theories in dense plasmas and may sparkle new theoretical developments, important for fundamental studies and applications in astrophysics and high-energy-density science.

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BibTeX
@article{condamine2026accessing,
  title = {{Accessing the fundamental link between atomic populations and frequency distribution of spectral lines of ions in dense plasmas}},
  author = {F. P. Condamine and E. Galtier and O. Renner and D. Khaghani and L. Gournay and P. Vachal and E. Cunningham and G. Dyer and M. Greenberg and B. Nagler and H.-J. Lee and S. H. Glenzer and J. P. Marques and Paul Indelicato and A. V. Demura and V. S. Lisitsa and L. A. Vainshtein and F. B. Rosmej},
  journal = {Communications Physics},
  year = {2026},
  month = aug,
  doi = {10.1038/s42005-026-02798-y},
  url = {https://hal.science/hal-05747080v1},
  note = {CC BY-NC-ND 4.0},
}
RIS
TY  - JOUR
TI  - Accessing the fundamental link between atomic populations and frequency distribution of spectral lines of ions in dense plasmas
AU  - F. P. Condamine
AU  - E. Galtier
AU  - O. Renner
AU  - D. Khaghani
AU  - L. Gournay
AU  - P. Vachal
AU  - E. Cunningham
AU  - G. Dyer
AU  - M. Greenberg
AU  - B. Nagler
AU  - H.-J. Lee
AU  - S. H. Glenzer
AU  - J. P. Marques
AU  - Paul Indelicato
AU  - A. V. Demura
AU  - V. S. Lisitsa
AU  - L. A. Vainshtein
AU  - F. B. Rosmej
PY  - 2026
DA  - 2026/08/20
JO  - Communications Physics
DO  - 10.1038/s42005-026-02798-y
UR  - https://hal.science/hal-05747080v1
AB  - Dense plasmas enable to test our fundamental understanding of matter but a lack of data hindered searches of new physics in the past. A game changer is the new and unique Stanford-Linear-Accelerator-Center allowing X-ray line-shape-resolved resonance pumping via a combination of the self-seeded Linac-Coherent-Light-Source beam with an optical-laser produced dense plasma: Non-isolated atom models can now be benchmarked via the spectral distribution. High-precision spectroscopy reveals significant and simultaneous redistribution in population and frequency for transitions in He-like Vanadium. A critical principal quantum number is identified above which a strong intensity enhancement of higher lying Rydberg-lines appears although the corresponding ionic levels are not directly pumped. The Rydberg-lines themselves show significant distortions of their spectral distribution. We determine their frequency distributions with a precision of 0.2eV at 6.6keV and observe significant systematic deviations from available numerical methods. Our data question the current understanding how local thermodynamic equilibrium can be achieved. They also serve as a crucial benchmark for quantum theories in dense plasmas and may sparkle new theoretical developments, important for fundamental studies and applications in astrophysics and high-energy-density science.
SN  - 2399-3650
SN  - 2399-3650
ER  -