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Correlation-Driven Nonlinear Magnetoelectric Response in an Altermagnet: A Dynamical Mean-Field Study

Abstract

We investigate the optical nonlinear magnetoelectric effect (NMEE) in a strongly correlated altermagnet using dynamical mean-field theory. Unlike effective band descriptions with an imposed spin splitting, our approach determines the altermagnetic order, electronic spectrum, and optical nonlinear response self-consistently. We find that the NMEE is finite in the altermagnetic phase and vanishes in the paramagnetic phase. Its frequency dependence reflects the spin-resolved spectral structure and provides an estimate of the characteristic altermagnetic spin-splitting scale. Interaction and temperature tuning produce qualitatively different behavior: at low temperature, reducing the interaction strength toward the interaction-driven magnetic phase boundary enhances the response, whereas increasing the temperature suppresses it and drives it to zero above the critical temperature. These results establish the optical NMEE as a probe of correlated altermagnetic order and suggest that tuning parameters such as pressure, strain, or chemical substitution toward an interaction-driven phase boundary may provide a promising route to maximizing the response.

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BibTeX
@misc{peters2026correlationdriven,
  title = {{Correlation-Driven Nonlinear Magnetoelectric Response in an Altermagnet: A Dynamical Mean-Field Study}},
  author = {Robert Peters and Jun Ōiké},
  howpublished = {arXiv},
  year = {2026},
  month = sep,
  doi = {10.48550/arxiv.2609.00697},
  eprint = {2609.00697},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2609.00697},
}
RIS
TY  - UNPB
TI  - Correlation-Driven Nonlinear Magnetoelectric Response in an Altermagnet: A Dynamical Mean-Field Study
AU  - Robert Peters
AU  - Jun Ōiké
PY  - 2026
DA  - 2026/09/01
PB  - arXiv
DO  - 10.48550/arxiv.2609.00697
UR  - https://arxiv.org/abs/2609.00697
AB  - We investigate the optical nonlinear magnetoelectric effect (NMEE) in a strongly correlated altermagnet using dynamical mean-field theory. Unlike effective band descriptions with an imposed spin splitting, our approach determines the altermagnetic order, electronic spectrum, and optical nonlinear response self-consistently. We find that the NMEE is finite in the altermagnetic phase and vanishes in the paramagnetic phase. Its frequency dependence reflects the spin-resolved spectral structure and provides an estimate of the characteristic altermagnetic spin-splitting scale. Interaction and temperature tuning produce qualitatively different behavior: at low temperature, reducing the interaction strength toward the interaction-driven magnetic phase boundary enhances the response, whereas increasing the temperature suppresses it and drives it to zero above the critical temperature. These results establish the optical NMEE as a probe of correlated altermagnetic order and suggest that tuning parameters such as pressure, strain, or chemical substitution toward an interaction-driven phase boundary may provide a promising route to maximizing the response.
ER  -