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PreprintarXiv licencearXiv

Sub-shot-noise mid-infrared photothermal measurements using twin beams

Abstract

Mid-infrared photothermal (MIP) measurement probes refractive-index changes induced by mid-infrared (MIR) absorption using visible or near-infrared light and has recently emerged as a powerful modality for MIR spectro-imaging in the life sciences. Reducing measurement noise allows the probe power to be lowered without compromising the signal-to-noise ratio (SNR), thereby mitigating the risk of sample damage. However, even in the absence of classical noise, the SNR of conventional MIP measurements using a classical coherent probe is fundamentally limited by shot noise. Here, we demonstrate sub-shot-noise MIP measurement using twin beams generated through seeded optical parametric amplification. Balanced detection of the twin beams suppresses the noise by more than 5 dB below the shot-noise level established using a coherent beam. As a proof-of-principle demonstration, we measure the MIP signal from liquid water using balanced twin-beam detection and achieve an SNR enhancement of more than 2 dB over the balanced coherent-beam detection.

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BibTeX
@misc{hashimoto2026subshotnoise,
  title = {{Sub-shot-noise mid-infrared photothermal measurements using twin beams}},
  author = {Kazuki Hashimoto and Takuro Ideguchi},
  howpublished = {arXiv},
  year = {2026},
  month = oct,
  doi = {10.48550/arxiv.2610.10294},
  eprint = {2610.10294},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2610.10294},
}
RIS
TY  - UNPB
TI  - Sub-shot-noise mid-infrared photothermal measurements using twin beams
AU  - Kazuki Hashimoto
AU  - Takuro Ideguchi
PY  - 2026
DA  - 2026/10/07
PB  - arXiv
DO  - 10.48550/arxiv.2610.10294
UR  - https://arxiv.org/abs/2610.10294
AB  - Mid-infrared photothermal (MIP) measurement probes refractive-index changes induced by mid-infrared (MIR) absorption using visible or near-infrared light and has recently emerged as a powerful modality for MIR spectro-imaging in the life sciences. Reducing measurement noise allows the probe power to be lowered without compromising the signal-to-noise ratio (SNR), thereby mitigating the risk of sample damage. However, even in the absence of classical noise, the SNR of conventional MIP measurements using a classical coherent probe is fundamentally limited by shot noise. Here, we demonstrate sub-shot-noise MIP measurement using twin beams generated through seeded optical parametric amplification. Balanced detection of the twin beams suppresses the noise by more than 5 dB below the shot-noise level established using a coherent beam. As a proof-of-principle demonstration, we measure the MIP signal from liquid water using balanced twin-beam detection and achieve an SNR enhancement of more than 2 dB over the balanced coherent-beam detection.
ER  -