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PreprintCC BY-NC-SA 4.0arXiv

μSR measurements of 3D Ising ferromagnetism in bulk Fe3GeTe2 crystals

Abstract

Fe3GeTe2 is a quasi-two-dimensional itinerant ferromagnet with a van-der-Waals layered structure that exhibits substantial magnetic anisotropy. In bulk samples, this material becomes magnetically ordered below 220~K, while in thin samples, the gate-tunability of the ferromagnetic moment has attracted significant interest. Alongside high-temperature ferromagnetism, a low-temperature magnetic state occurs whose nature has not been conclusively identified, with some studies suggesting a transition between ferromagnetism and antiferromagnetism with temperature. Here we present magnetometry and μSR data that demonstrate that Fe3GeTe2 exhibits three-dimenional Ising-like ferromagnetism over the entire temperature range between TC=220~K and 2~K. The feature at 170~K that has previously been proposed to be a transition to antiferromagnetism is instead likely to represent a domain-freezing transition.

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BibTeX
@misc{wilson2026μsr,
  title = {{$μ$SR measurements of 3D Ising ferromagnetism in bulk Fe$_3$GeTe$_2$ crystals}},
  author = {M. N. Wilson and J. Huang and T. J. Hicken and D. A. Mayoh and B. M. Huddart and G. Balakrishnan and T. Lancaster},
  howpublished = {arXiv},
  year = {2026},
  month = sep,
  doi = {10.48550/arxiv.2609.39806},
  eprint = {2609.39806},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2609.39806},
  note = {CC BY-NC-SA 4.0},
}
RIS
TY  - UNPB
TI  - μSR measurements of 3D Ising ferromagnetism in bulk Fe_3GeTe_2 crystals
AU  - M. N. Wilson
AU  - J. Huang
AU  - T. J. Hicken
AU  - D. A. Mayoh
AU  - B. M. Huddart
AU  - G. Balakrishnan
AU  - T. Lancaster
PY  - 2026
DA  - 2026/09/30
PB  - arXiv
DO  - 10.48550/arxiv.2609.39806
UR  - https://arxiv.org/abs/2609.39806
AB  - Fe_3GeTe_2 is a quasi-two-dimensional itinerant ferromagnet with a van-der-Waals layered structure that exhibits substantial magnetic anisotropy. In bulk samples, this material becomes magnetically ordered below 220~K, while in thin samples, the gate-tunability of the ferromagnetic moment has attracted significant interest. Alongside high-temperature ferromagnetism, a low-temperature magnetic state occurs whose nature has not been conclusively identified, with some studies suggesting a transition between ferromagnetism and antiferromagnetism with temperature. Here we present magnetometry and μSR data that demonstrate that Fe_3GeTe_2 exhibits three-dimenional Ising-like ferromagnetism over the entire temperature range between T_C=220~K and 2~K. The feature at 170~K that has previously been proposed to be a transition to antiferromagnetism is instead likely to represent a domain-freezing transition.
ER  -