Theory of extrinsic contributions to the full orbital current
Abstract
The orbital Hall effect (OHE) underpins the emerging field of orbitronics. A complete quantum-mechanical evaluation of the usual orbital-current operator must retain all matrix elements of the position operator, including its band-diagonal differential part; intrinsic calculations based on this full evaluation can differ by orders of magnitude from the conventional truncation. A relaxation-time estimate of disorder effects on the full current has been reported, but a microscopic treatment of extrinsic scattering has remained unavailable because the position operator requires wavevector-off-diagonal density-matrix elements. Here we develop such a theory by solving the quantum kinetic equation for the wavevector-off-diagonal density matrix, including band-structure, field-corrected side-jump, and skew-scattering terms within the non-crossing approximation. We apply the theory to a massive Dirac cone and to the same model with a particle-hole-symmetry-breaking quadratic term. Disorder-generated contributions of order τ0 are generically comparable to the intrinsic current in the metallic regime and cannot be separated from it by simple disorder-strength scaling. For the bare massive Dirac cone the surviving non-crossing extrinsic correction cancels the conventional intrinsic value and leaves a total current exactly twice the quantum correction, whereas particle-hole asymmetry activates conventional skew scattering for disorder with a non-zero third moment, which dominates in sufficiently clean samples. The wavevector-off-diagonal construction is independent of the two-band model and provides a general route to disorder corrections for position-dependent observables in multiband solids.
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BibTeX
@misc{cullen2026theory,
title = {{Theory of extrinsic contributions to the full orbital current}},
author = {James H Cullen and Dimitrie Culcer},
howpublished = {arXiv},
year = {2026},
month = sep,
doi = {10.48550/arxiv.2609.28628},
eprint = {2609.28628},
archivePrefix = {arXiv},
url = {https://arxiv.org/abs/2609.28628},
}
RIS
TY - UNPB
TI - Theory of extrinsic contributions to the full orbital current
AU - James H Cullen
AU - Dimitrie Culcer
PY - 2026
DA - 2026/09/23
PB - arXiv
DO - 10.48550/arxiv.2609.28628
UR - https://arxiv.org/abs/2609.28628
AB - The orbital Hall effect (OHE) underpins the emerging field of orbitronics. A complete quantum-mechanical evaluation of the usual orbital-current operator must retain all matrix elements of the position operator, including its band-diagonal differential part; intrinsic calculations based on this full evaluation can differ by orders of magnitude from the conventional truncation. A relaxation-time estimate of disorder effects on the full current has been reported, but a microscopic treatment of extrinsic scattering has remained unavailable because the position operator requires wavevector-off-diagonal density-matrix elements. Here we develop such a theory by solving the quantum kinetic equation for the wavevector-off-diagonal density matrix, including band-structure, field-corrected side-jump, and skew-scattering terms within the non-crossing approximation. We apply the theory to a massive Dirac cone and to the same model with a particle-hole-symmetry-breaking quadratic term. Disorder-generated contributions of order τ^0 are generically comparable to the intrinsic current in the metallic regime and cannot be separated from it by simple disorder-strength scaling. For the bare massive Dirac cone the surviving non-crossing extrinsic correction cancels the conventional intrinsic value and leaves a total current exactly twice the quantum correction, whereas particle-hole asymmetry activates conventional skew scattering for disorder with a non-zero third moment, which dominates in sufficiently clean samples. The wavevector-off-diagonal construction is independent of the two-band model and provides a general route to disorder corrections for position-dependent observables in multiband solids.
ER -