Imaging atomic-scale surface structure and superconducting gap of the misfit layered compound (SnS)1.17NbS2
Abstract
Superlattices of van der Waals-coupled two-dimensional materials offer a platform for engineering electronic band structure and fostering emergent quantum states. Misfit layered compounds provide naturally assembled superlattices, in which crystallographically distinct two-dimensional subsystems coexist within a single bulk crystal. Therein, the presence of both commensurate and incommensurate lattice directions introduces structural modulation, which might alter real-space electronic orders such as superconductivity. Here, we investigate the atomic-scale surface structure and local superconductivity of the misfit layered compound (SnS)1.17NbS2 using structural characterization, electrical transport, and low-temperature scanning tunnelling microscopy (STM). While X-ray diffraction and cross-sectional scanning transmission electron microscopy confirm the bulk misfit structure, STM resolves large SnS- and NbS2-terminated terraces, where the surface atomic registry differs from the bulk misfit structure. Furthermore, tunnelling spectroscopy at 2 K reveals nearly identical superconducting gaps on both terminations, and the spatial variation of the gap shows no visible modulation that corresponds to the misfit lattice. These results establish an atomic-scale picture of the surface structure and superconducting states of this naturally assembled misfit heterostructure.
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BibTeX
@misc{zhao2026imaging,
title = {{Imaging atomic-scale surface structure and superconducting gap of the misfit layered compound (SnS)1.17NbS2}},
author = {Dongming Zhao and Shamarita Deb and Lichen Ji and Souvik Das and Paul Simon and Raúl Cardoso-Gil and Steffen Wirth and Walter Schnelle and Sushmita Chandra and Jian-Feng Ge and Claudia Felser},
howpublished = {arXiv},
year = {2026},
month = oct,
doi = {10.48550/arxiv.2610.17879},
eprint = {2610.17879},
archivePrefix = {arXiv},
url = {https://arxiv.org/abs/2610.17879},
note = {CC BY 4.0},
}
RIS
TY - UNPB
TI - Imaging atomic-scale surface structure and superconducting gap of the misfit layered compound (SnS)1.17NbS2
AU - Dongming Zhao
AU - Shamarita Deb
AU - Lichen Ji
AU - Souvik Das
AU - Paul Simon
AU - Raúl Cardoso-Gil
AU - Steffen Wirth
AU - Walter Schnelle
AU - Sushmita Chandra
AU - Jian-Feng Ge
AU - Claudia Felser
PY - 2026
DA - 2026/10/13
PB - arXiv
DO - 10.48550/arxiv.2610.17879
UR - https://arxiv.org/abs/2610.17879
AB - Superlattices of van der Waals-coupled two-dimensional materials offer a platform for engineering electronic band structure and fostering emergent quantum states. Misfit layered compounds provide naturally assembled superlattices, in which crystallographically distinct two-dimensional subsystems coexist within a single bulk crystal. Therein, the presence of both commensurate and incommensurate lattice directions introduces structural modulation, which might alter real-space electronic orders such as superconductivity. Here, we investigate the atomic-scale surface structure and local superconductivity of the misfit layered compound (SnS)1.17NbS2 using structural characterization, electrical transport, and low-temperature scanning tunnelling microscopy (STM). While X-ray diffraction and cross-sectional scanning transmission electron microscopy confirm the bulk misfit structure, STM resolves large SnS- and NbS2-terminated terraces, where the surface atomic registry differs from the bulk misfit structure. Furthermore, tunnelling spectroscopy at 2 K reveals nearly identical superconducting gaps on both terminations, and the spatial variation of the gap shows no visible modulation that corresponds to the misfit lattice. These results establish an atomic-scale picture of the surface structure and superconducting states of this naturally assembled misfit heterostructure.
ER -