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PreprintarXiv licencearXiv

Altermagnetism-Induced Spin-resolved electronic structure in Janus FeX0.5Y0.5 Monolayers (X, Y = S, Se, Te)

Abstract

Realizing the spin-resolved electronic properties in superconducting materials stands as a critical frontier, offering both novel fundamental physics and potential for dissipationless spin-based devices. Here, we predict a series of Janus FeX0.5Y0.5 monolayers derived from iron-based superconductors (e.g., FeSe, FeTe, and FeS) by using Kondo-type model and first-principles calculations. These Janus structures exhibit significant spin-splittingelectronic states, large topological band gaps (51.4 meV) and high Néel temperatures (415 K). We further reveal that valley polarization can be effectively tuned via applied in-plane strain and the resulting valley-polarized anomalous Hall conductivity can be manipulated by shifting the Fermi level. Our work suggests a new strategy based on altermagnetism for engineering spin-splitting states in superconducting systems and inspires further exploration of superconducting spintronics.

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BibTeX
@misc{zhang2026altermagnetisminduced,
  title = {{Altermagnetism-Induced Spin-resolved electronic structure in Janus FeX0.5Y0.5 Monolayers (X, Y = S, Se, Te)}},
  author = {Mengyang Zhang and Jie Li and Yifei Chen and Shifang Li and Zhentao Fu and Jianxin Zhong},
  howpublished = {arXiv},
  year = {2026},
  month = oct,
  doi = {10.48550/arxiv.2608.09054},
  eprint = {2608.09054},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2608.09054},
}
RIS
TY  - UNPB
TI  - Altermagnetism-Induced Spin-resolved electronic structure in Janus FeX0.5Y0.5 Monolayers (X, Y = S, Se, Te)
AU  - Mengyang Zhang
AU  - Jie Li
AU  - Yifei Chen
AU  - Shifang Li
AU  - Zhentao Fu
AU  - Jianxin Zhong
PY  - 2026
DA  - 2026/10/14
PB  - arXiv
DO  - 10.48550/arxiv.2608.09054
UR  - https://arxiv.org/abs/2608.09054
AB  - Realizing the spin-resolved electronic properties in superconducting materials stands as a critical frontier, offering both novel fundamental physics and potential for dissipationless spin-based devices. Here, we predict a series of Janus FeX0.5Y0.5 monolayers derived from iron-based superconductors (e.g., FeSe, FeTe, and FeS) by using Kondo-type model and first-principles calculations. These Janus structures exhibit significant spin-splittingelectronic states, large topological band gaps (51.4 meV) and high Néel temperatures (415 K). We further reveal that valley polarization can be effectively tuned via applied in-plane strain and the resulting valley-polarized anomalous Hall conductivity can be manipulated by shifting the Fermi level. Our work suggests a new strategy based on altermagnetism for engineering spin-splitting states in superconducting systems and inspires further exploration of superconducting spintronics.
ER  -