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Results on 235U(nth,f) isotopic fission yields using prompt and delayed gamma rays at the FIPPS spectrometer of the ILL

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Abstract

We present preliminary results from a measurement campaign conducted with the FIPPS γ-ray spectrometer at the ILL using an active target made of 235U dissolved in a liquid scintillator. Prompt γ rays were used to extract absolute, independent isotopic fission yields. We obtained yields for a selected set of well-produced even-even nuclei from the 235U(nth,f) reaction and compared them with JEFF-3.3 evaluated data. This included the doubly magic nucleus 132Sn, for which we observed a pronounced deficit (about a factor 7) with respect to JEFF-3.3. Using the FIFRELIN fission fragment de-excitation code, we interpreted this discrepancy as evidence that 132Sn is mainly produced in its ground state at scission or after neutron evaporation. Delayed γ rays recorded in the same experiment were also analysed. No deviation was found in the beta decay of 132Sn compared to the nuclear database. However, an excess of about a 40% was found in the β decay of 90Kr, which may originate from an overestimated ground-state feeding of 90Rb in the evaluated data.

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BibTeX
@misc{materna2026results,
  title = {{Results on $^235$U(n$_\mathrmth$,f) isotopic fission yields using prompt and delayed gamma rays at the FIPPS spectrometer of the ILL}},
  author = {T Materna and P Herran and M Ballu and Q Poirier and A Letourneau and D Doré and L Thulliez and C Michelagnoli and F Kandzia and Y.H Kim and U Köster and O Litaize and O Sérot and A Chebboubi},
  howpublished = {HAL},
  year = {2026},
  month = sep,
  doi = {10.48550/arxiv.2609.13033},
  eprint = {2609.13033},
  archivePrefix = {arXiv},
  url = {https://hal.science/hal-05771266v1},
  note = {CC BY-NC-ND 4.0},
}
RIS
TY  - UNPB
TI  - Results on ^235U(n_th,f) isotopic fission yields using prompt and delayed gamma rays at the FIPPS spectrometer of the ILL
AU  - T Materna
AU  - P Herran
AU  - M Ballu
AU  - Q Poirier
AU  - A Letourneau
AU  - D Doré
AU  - L Thulliez
AU  - C Michelagnoli
AU  - F Kandzia
AU  - Y.H Kim
AU  - U Köster
AU  - O Litaize
AU  - O Sérot
AU  - A Chebboubi
PY  - 2026
DA  - 2026/09/11
PB  - HAL
DO  - 10.48550/arxiv.2609.13033
UR  - https://hal.science/hal-05771266v1
AB  - We present preliminary results from a measurement campaign conducted with the FIPPS γ-ray spectrometer at the ILL using an active target made of ^235U dissolved in a liquid scintillator. Prompt γ rays were used to extract absolute, independent isotopic fission yields. We obtained yields for a selected set of well-produced even-even nuclei from the ^235U(n_th,f) reaction and compared them with JEFF-3.3 evaluated data. This included the doubly magic nucleus ^132Sn, for which we observed a pronounced deficit (about a factor 7) with respect to JEFF-3.3. Using the FIFRELIN fission fragment de-excitation code, we interpreted this discrepancy as evidence that ^132Sn is mainly produced in its ground state at scission or after neutron evaporation. Delayed γ rays recorded in the same experiment were also analysed. No deviation was found in the beta decay of ^132Sn compared to the nuclear database. However, an excess of about a 40% was found in the β decay of ^90Kr, which may originate from an overestimated ground-state feeding of ^90Rb in the evaluated data.
ER  -