Relative roles of aerosol size and hygroscopicity in modulating marine liquid-phase cloud responses under the winter monsoon
- 1Nanjing University of Information Science and Technology (Nanjing, China)
Abstract
How aerosol physicochemical properties affect aerosol-cloud interactions (ACI) and when these impacts are most pronounced represent an important source of ACI uncertainty. Targeting a representative liquid-phase cloud case over the Eastern China Ocean (ECO) under the winter monsoon featuring abundant meteorological, aerosol, and cloud variations, this study investigates the impacts of changes in aerosol size (volume-mean radius increased by 1.2 times and decreased by 45 %) and hygroscopicity (volume-mean hygroscopicity increased by 2.2 times and decreased by 62 %) using a spectral-bin cloud model. Results indicate that increased aerosol size and hygroscopicity generally enhance cloud development, raising the averaged cloud droplet number concentration ( N d ) by 92 % and 53 %, respectively. These impacts peak under moderate aerosol concentrations ( N a ) and cold advection, where N d increases up to 10-fold. Concurrently, increased aerosol size raises cloud water by 1.3 times and extends cloud lifetime by 85 %, whereas increased hygroscopicity has a much weaker effect. By contrast, decreased aerosol size and hygroscopicity generally suppress cloud development, reducing the averaged N d by 49 % and 43 %, respectively. The former has a relatively strong impact, which is most notable in moderate-to-high N a environments under cold advection, reducing N d and cloud water by over 80 % and 50 %, respectively. While changes in aerosol size generally exert a stronger overall impact than changes in hygroscopicity, specific conditions reveal the opposite. Notably, the enhancement of N d by increased hygroscopicity under high N a , and the preservation of cloud and rainwater through evaporation suppression by decreased hygroscopicity, both surpass the effects caused by corresponding aerosol size changes.
Versions
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BibTeX
@article{zhao2026relative,
title = {{Relative roles of aerosol size and hygroscopicity in modulating marine liquid-phase cloud responses under the winter monsoon}},
author = {Jianqi Zhao and Xiaoyan Ma and Hailing Jia and Tong Yang and Peili Zou and Yingying Ku},
journal = {Atmospheric Chemistry and Physics},
year = {2026},
month = oct,
doi = {10.5194/acp-26-15117-2026},
url = {https://doi.org/10.5194/acp-26-15117-2026},
note = {CC BY 4.0},
}
RIS
TY - JOUR
TI - Relative roles of aerosol size and hygroscopicity in modulating marine liquid-phase cloud responses under the winter monsoon
AU - Jianqi Zhao
AU - Xiaoyan Ma
AU - Hailing Jia
AU - Tong Yang
AU - Peili Zou
AU - Yingying Ku
PY - 2026
DA - 2026/10/28
JO - Atmospheric Chemistry and Physics
DO - 10.5194/acp-26-15117-2026
UR - https://doi.org/10.5194/acp-26-15117-2026
AB - How aerosol physicochemical properties affect aerosol-cloud interactions (ACI) and when these impacts are most pronounced represent an important source of ACI uncertainty. Targeting a representative liquid-phase cloud case over the Eastern China Ocean (ECO) under the winter monsoon featuring abundant meteorological, aerosol, and cloud variations, this study investigates the impacts of changes in aerosol size (volume-mean radius increased by 1.2 times and decreased by 45 %) and hygroscopicity (volume-mean hygroscopicity increased by 2.2 times and decreased by 62 %) using a spectral-bin cloud model. Results indicate that increased aerosol size and hygroscopicity generally enhance cloud development, raising the averaged cloud droplet number concentration ( N d ) by 92 % and 53 %, respectively. These impacts peak under moderate aerosol concentrations ( N a ) and cold advection, where N d increases up to 10-fold. Concurrently, increased aerosol size raises cloud water by 1.3 times and extends cloud lifetime by 85 %, whereas increased hygroscopicity has a much weaker effect. By contrast, decreased aerosol size and hygroscopicity generally suppress cloud development, reducing the averaged N d by 49 % and 43 %, respectively. The former has a relatively strong impact, which is most notable in moderate-to-high N a environments under cold advection, reducing N d and cloud water by over 80 % and 50 %, respectively. While changes in aerosol size generally exert a stronger overall impact than changes in hygroscopicity, specific conditions reveal the opposite. Notably, the enhancement of N d by increased hygroscopicity under high N a , and the preservation of cloud and rainwater through evaporation suppression by decreased hygroscopicity, both surpass the effects caused by corresponding aerosol size changes.
SN - 1680-7324
ER -