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Peer-reviewedCC BY 4.0Communications Physics

Hierarchical structure of primary and hybridization-induced superconducting correlations in bilayer nickelates

Abstract

The discovery of high-pressure superconductivity in the bilayer nickelate La ₃ Ni ₂ O ₇ , with a transition temperature approaching 80 K, has stimulated intense debate regarding its microscopic origin. Although an s ± gap symmetry has been widely proposed, the electronic degrees of freedom responsible for pairing remain unsettled. Here we investigate a bilayer two-orbital Hubbard model using the variational Monte Carlo method and reveal a hierarchical pairing structure in bilayer nickelates. The primary pairing tendency originates from the bonding–antibonding splitting of the Ni 3dz2 3 d z 2 orbitals, while orbital hybridization redistributes superconducting correlations to the dx2−y2 d x 2 − y 2 channel despite its weak intrinsic pairing tendency. This distinction between the origin of pairing and the resulting superconducting correlations explains why the two orbital channels exhibit comparable long-range correlations. The resulting s ± state is robust against changes in Fermi-surface topology. These results reconcile apparently competing theoretical scenarios and provide a comprehensive understanding, highlighting the distinctive role of orbital hybridization in multilayer correlated superconductors.

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BibTeX
@article{watanabe2026hierarchical,
  title = {{Hierarchical structure of primary and hybridization-induced superconducting correlations in bilayer nickelates}},
  author = {Hiroshi Watanabe and Hirofumi Sakakibara and Kazuhiko Kuroki},
  journal = {Communications Physics},
  year = {2026},
  month = oct,
  doi = {10.1038/s42005-026-02928-6},
  url = {https://www.nature.com/articles/s42005-026-02928-6},
  note = {CC BY 4.0},
}
RIS
TY  - JOUR
TI  - Hierarchical structure of primary and hybridization-induced superconducting correlations in bilayer nickelates
AU  - Hiroshi Watanabe
AU  - Hirofumi Sakakibara
AU  - Kazuhiko Kuroki
PY  - 2026
DA  - 2026/10/28
JO  - Communications Physics
DO  - 10.1038/s42005-026-02928-6
UR  - https://www.nature.com/articles/s42005-026-02928-6
AB  - The discovery of high-pressure superconductivity in the bilayer nickelate La ₃ Ni ₂ O ₇ , with a transition temperature approaching 80 K, has stimulated intense debate regarding its microscopic origin. Although an s ± gap symmetry has been widely proposed, the electronic degrees of freedom responsible for pairing remain unsettled. Here we investigate a bilayer two-orbital Hubbard model using the variational Monte Carlo method and reveal a hierarchical pairing structure in bilayer nickelates. The primary pairing tendency originates from the bonding–antibonding splitting of the Ni 3d_z^2 3 d z 2 orbitals, while orbital hybridization redistributes superconducting correlations to the d_x^2−y^2 d x 2 − y 2 channel despite its weak intrinsic pairing tendency. This distinction between the origin of pairing and the resulting superconducting correlations explains why the two orbital channels exhibit comparable long-range correlations. The resulting s ± state is robust against changes in Fermi-surface topology. These results reconcile apparently competing theoretical scenarios and provide a comprehensive understanding, highlighting the distinctive role of orbital hybridization in multilayer correlated superconductors.
SN  - 2399-3650
ER  -