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PreprintCC BY 4.0arXiv

Non-magnetic impurities as a quantum microscope of finite size effects in spin chains

Abstract

Finite-size effects are ubiquitous in quantum matter, yet typically invisible in the thermodynamic limit; when system size is restricted, boundaries and confinement reveal modified spectra, correlations, and emergent phenomena. With growing access to well-controlled few-spin systems, these effects are now directly observable and offer a route to probing universal physics and enabling quantum information applications. Here, we study finite-size physics in the quasi-one-dimensional Ising-like quantum antiferromagnet Ba(Co1−xMgx)2V2O8 with x = 2% and x = 5%, where non-magnetic Mg2+ ions fragment the Co2+ spin chains into finite segments. Combining inelastic neutron scattering and numerical calculations, we identify distinct regimes with fundamentally different low-energy quantum excitations: spinons confined to chain boundaries, and a cluster mode in shorter chains corresponding to a collective reversal of the Néel-ordered segment without classical analogue. Our results demonstrate how chemical substitution acts as a quantum microscope providing direct access to boundary-shaped excitations in strongly correlated spin systems.

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BibTeX
@misc{faure2026nonmagnetic,
  title = {{Non-magnetic impurities as a quantum microscope of finite size effects in spin chains}},
  author = {Quentin Faure and Shintaro Takayoshi and Virginie Simonet and Béatrice Grenier and Stéphane Raymond and Eric Ressouche and Xavier Fabrèges and Pascal Lejay and Thierry Giamarchi and Sylvain Petit},
  howpublished = {arXiv},
  year = {2026},
  month = oct,
  doi = {10.48550/arxiv.2610.34596},
  eprint = {2610.34596},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2610.34596},
  note = {CC BY 4.0},
}
RIS
TY  - UNPB
TI  - Non-magnetic impurities as a quantum microscope of finite size effects in spin chains
AU  - Quentin Faure
AU  - Shintaro Takayoshi
AU  - Virginie Simonet
AU  - Béatrice Grenier
AU  - Stéphane Raymond
AU  - Eric Ressouche
AU  - Xavier Fabrèges
AU  - Pascal Lejay
AU  - Thierry Giamarchi
AU  - Sylvain Petit
PY  - 2026
DA  - 2026/10/25
PB  - arXiv
DO  - 10.48550/arxiv.2610.34596
UR  - https://arxiv.org/abs/2610.34596
AB  - Finite-size effects are ubiquitous in quantum matter, yet typically invisible in the thermodynamic limit; when system size is restricted, boundaries and confinement reveal modified spectra, correlations, and emergent phenomena. With growing access to well-controlled few-spin systems, these effects are now directly observable and offer a route to probing universal physics and enabling quantum information applications. Here, we study finite-size physics in the quasi-one-dimensional Ising-like quantum antiferromagnet Ba(Co_1−xMg_x)_2V_2O_8 with x = 2% and x = 5%, where non-magnetic Mg^2+ ions fragment the Co^2+ spin chains into finite segments. Combining inelastic neutron scattering and numerical calculations, we identify distinct regimes with fundamentally different low-energy quantum excitations: spinons confined to chain boundaries, and a cluster mode in shorter chains corresponding to a collective reversal of the Néel-ordered segment without classical analogue. Our results demonstrate how chemical substitution acts as a quantum microscope providing direct access to boundary-shaped excitations in strongly correlated spin systems.
ER  -