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PreprintarXiv licencearXiv

Flaw-tolerant recycling of waste tires into high-performance rubber

Abstract

Annually about one billion tires reach the end of life. Rubber from waste tires can be ground into particles and incorporated into a matrix. In practice, the resulting composites are commonly not recycled into new tires, but downcycled into low-value products such as sport surfaces, indoor flooring, and rubberized asphalt. Recycling waste tires into new tires remains a challenge. In particular, such composites typically have low strength, especially when the particle content is high or the particles are large. A single waste tire particle may act as a flaw to initiate macroscopic fracture and knock down the strength of the entire composite. Here we propose the principle of flaw-tolerant recycling. Rather than requiring every particle to be reliable and small, the matrix is designed so that flaw-like particles do not initiate macroscopic fracture. We demonstrate a flaw-tolerant matrix consisting of two intertwined networks: a network of densely entangled and sparsely crosslinked long natural rubber chains, and a percolated network of carbon aggregates. When the flaw-tolerant matrix is incorporated with up to 80 wt% of commercially available waste particles, the resulting composites still maintain strength. The principle of flaw-tolerant recycling may aid the development of recycling waste tires into new tires.

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BibTeX
@misc{li2026flawtolerant,
  title = {{Flaw-tolerant recycling of waste tires into high-performance rubber}},
  author = {Chenghai Li and Yu Zhou and Zheqi Chen and Jun Ho Min and Matthew Wei Ming Tan and Masako Yoshihara Yang and Yakov Kutsovsky and Zhigang Suo},
  howpublished = {arXiv},
  year = {2026},
  month = oct,
  doi = {10.48550/arxiv.2610.25572},
  eprint = {2610.25572},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2610.25572},
}
RIS
TY  - UNPB
TI  - Flaw-tolerant recycling of waste tires into high-performance rubber
AU  - Chenghai Li
AU  - Yu Zhou
AU  - Zheqi Chen
AU  - Jun Ho Min
AU  - Matthew Wei Ming Tan
AU  - Masako Yoshihara Yang
AU  - Yakov Kutsovsky
AU  - Zhigang Suo
PY  - 2026
DA  - 2026/10/18
PB  - arXiv
DO  - 10.48550/arxiv.2610.25572
UR  - https://arxiv.org/abs/2610.25572
AB  - Annually about one billion tires reach the end of life. Rubber from waste tires can be ground into particles and incorporated into a matrix. In practice, the resulting composites are commonly not recycled into new tires, but downcycled into low-value products such as sport surfaces, indoor flooring, and rubberized asphalt. Recycling waste tires into new tires remains a challenge. In particular, such composites typically have low strength, especially when the particle content is high or the particles are large. A single waste tire particle may act as a flaw to initiate macroscopic fracture and knock down the strength of the entire composite. Here we propose the principle of flaw-tolerant recycling. Rather than requiring every particle to be reliable and small, the matrix is designed so that flaw-like particles do not initiate macroscopic fracture. We demonstrate a flaw-tolerant matrix consisting of two intertwined networks: a network of densely entangled and sparsely crosslinked long natural rubber chains, and a percolated network of carbon aggregates. When the flaw-tolerant matrix is incorporated with up to 80 wt% of commercially available waste particles, the resulting composites still maintain strength. The principle of flaw-tolerant recycling may aid the development of recycling waste tires into new tires.
ER  -