Thermodynamic Evidence for Multiple Field-Induced Phases in an Anisotropic Kagome Antiferromagnet
Abstract
Kagome antiferromagnets are predicted to host exotic field-induced phases, yet experimental identification of their thermodynamic signatures remains challenging. Here we combine specific heat (C) and ultrasound measurements up to 36 T and down to 0.5 K to map the H−T phase diagram of the anisotropic kagome magnet Y3Cu9(OH)19Cl8. We show that the suppression of long-range antiferromagnetic order with field at ∼ 15 T approximately coincides with the onset of the unconventional 1/6 (or 1/9) magnetization plateau previously observed in this system. The attenuation (and sound velocity) then intriguingly increases down to 0.5 K just at μ0H = 15 T, and C/T becomes temperature independent. Moreover, our measurements are consistent with the opening of a spin gap Δ0≃3.5± 0.3 K within the plateau and reveal a further compressible (ungapped) phase beyond the plateau phase, unveiling a rich sequence of field-induced phases in this quantum magnet.
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BibTeX
@misc{schuchard2026thermodynamic,
title = {{Thermodynamic Evidence for Multiple Field-Induced Phases in an Anisotropic Kagome Antiferromagnet}},
author = {M. Schuchard and Q. Barthélemy and C. Marcenat and N. Wack and P. Puphal and A. De Muer and D. LeBoeuf and T. Klein},
howpublished = {arXiv},
year = {2026},
month = nov,
doi = {10.48550/arxiv.2611.04675},
eprint = {2611.04675},
archivePrefix = {arXiv},
url = {https://arxiv.org/abs/2611.04675},
note = {CC BY-SA 4.0},
}
RIS
TY - UNPB
TI - Thermodynamic Evidence for Multiple Field-Induced Phases in an Anisotropic Kagome Antiferromagnet
AU - M. Schuchard
AU - Q. Barthélemy
AU - C. Marcenat
AU - N. Wack
AU - P. Puphal
AU - A. De Muer
AU - D. LeBoeuf
AU - T. Klein
PY - 2026
DA - 2026/11/03
PB - arXiv
DO - 10.48550/arxiv.2611.04675
UR - https://arxiv.org/abs/2611.04675
AB - Kagome antiferromagnets are predicted to host exotic field-induced phases, yet experimental identification of their thermodynamic signatures remains challenging. Here we combine specific heat (C) and ultrasound measurements up to 36 T and down to 0.5 K to map the H−T phase diagram of the anisotropic kagome magnet Y_3Cu_9(OH)_19Cl_8. We show that the suppression of long-range antiferromagnetic order with field at ∼ 15 T approximately coincides with the onset of the unconventional 1/6 (or 1/9) magnetization plateau previously observed in this system. The attenuation (and sound velocity) then intriguingly increases down to 0.5 K just at μ_0H = 15 T, and C/T becomes temperature independent. Moreover, our measurements are consistent with the opening of a spin gap Δ_0≃3.5± 0.3 K within the plateau and reveal a further compressible (ungapped) phase beyond the plateau phase, unveiling a rich sequence of field-induced phases in this quantum magnet.
ER -