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PreprintCC BY-SA 4.0arXiv

Thermodynamic Evidence for Multiple Field-Induced Phases in an Anisotropic Kagome Antiferromagnet

Abstract

Kagome antiferromagnets are predicted to host exotic field-induced phases, yet experimental identification of their thermodynamic signatures remains challenging. Here we combine specific heat (C) and ultrasound measurements up to 36 T and down to 0.5 K to map the H−T phase diagram of the anisotropic kagome magnet Y3Cu9(OH)19Cl8. We show that the suppression of long-range antiferromagnetic order with field at ∼ 15 T approximately coincides with the onset of the unconventional 1/6 (or 1/9) magnetization plateau previously observed in this system. The attenuation (and sound velocity) then intriguingly increases down to 0.5 K just at μ0H = 15 T, and C/T becomes temperature independent. Moreover, our measurements are consistent with the opening of a spin gap Δ0≃3.5± 0.3 K within the plateau and reveal a further compressible (ungapped) phase beyond the plateau phase, unveiling a rich sequence of field-induced phases in this quantum magnet.

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BibTeX
@misc{schuchard2026thermodynamic,
  title = {{Thermodynamic Evidence for Multiple Field-Induced Phases in an Anisotropic Kagome Antiferromagnet}},
  author = {M. Schuchard and Q. Barthélemy and C. Marcenat and N. Wack and P. Puphal and A. De Muer and D. LeBoeuf and T. Klein},
  howpublished = {arXiv},
  year = {2026},
  month = nov,
  doi = {10.48550/arxiv.2611.04675},
  eprint = {2611.04675},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2611.04675},
  note = {CC BY-SA 4.0},
}
RIS
TY  - UNPB
TI  - Thermodynamic Evidence for Multiple Field-Induced Phases in an Anisotropic Kagome Antiferromagnet
AU  - M. Schuchard
AU  - Q. Barthélemy
AU  - C. Marcenat
AU  - N. Wack
AU  - P. Puphal
AU  - A. De Muer
AU  - D. LeBoeuf
AU  - T. Klein
PY  - 2026
DA  - 2026/11/03
PB  - arXiv
DO  - 10.48550/arxiv.2611.04675
UR  - https://arxiv.org/abs/2611.04675
AB  - Kagome antiferromagnets are predicted to host exotic field-induced phases, yet experimental identification of their thermodynamic signatures remains challenging. Here we combine specific heat (C) and ultrasound measurements up to 36 T and down to 0.5 K to map the H−T phase diagram of the anisotropic kagome magnet Y_3Cu_9(OH)_19Cl_8. We show that the suppression of long-range antiferromagnetic order with field at ∼ 15 T approximately coincides with the onset of the unconventional 1/6 (or 1/9) magnetization plateau previously observed in this system. The attenuation (and sound velocity) then intriguingly increases down to 0.5 K just at μ_0H = 15 T, and C/T becomes temperature independent. Moreover, our measurements are consistent with the opening of a spin gap Δ_0≃3.5± 0.3 K within the plateau and reveal a further compressible (ungapped) phase beyond the plateau phase, unveiling a rich sequence of field-induced phases in this quantum magnet.
ER  -