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PreprintCC BY 4.0arXiv

Breathers in solitonic room-temperature superlattice-induced superfluorescence in quasi-2D perovskites

Abstract

Recently, a soliton mechanism for room-temperature superfluorescence in thin perovskite films has been proposed, with a fundamental soliton predicted to remain stable under LO phonon--exciton interactions. At the same time, superlattice architectures offer a route to enhancing superfluorescence in perovskites. Motivated by recent observations of room-temperature superfluorescence in periodic superlattices of quasi-2D metal-halide perovskites, we extend the 2D nonlocal nonlinear Schrödinger equation describing Wannier exciton--LO phonon interactions to superlattice structures, obtaining a 3D nonlocal nonlinear Schrödinger equation. We show that interlayer tunnelling gives rise to breather dynamics corresponding to a stable fundamental soliton in mixed coordinate--momentum space, with the coordinate parallel to the layers and the momentum perpendicular to them. The breather dynamics originate from miniband formation, which induces a momentum-dependent phase modulation of the soliton. In the absence of interlayer tunnelling, the breather dynamics disappear and the soliton becomes stationary. These results establish a direct connection between interlayer tunnelling, miniband formation and soliton dynamics, suggesting that breather behavior can provide a signature of interlayer tunnelling in quasi-2D perovskite superlattices.

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BibTeX
@misc{gladkij2026breathers,
  title = {{Breathers in solitonic room-temperature superlattice-induced superfluorescence in quasi-2D perovskites}},
  author = {A. A. Gladkij and N. N. Rosanov and B. D. Fainberg},
  howpublished = {arXiv},
  year = {2026},
  month = sep,
  doi = {10.48550/arxiv.2609.08513},
  eprint = {2609.08513},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2609.08513},
  note = {CC BY 4.0},
}
RIS
TY  - UNPB
TI  - Breathers in solitonic room-temperature superlattice-induced superfluorescence in quasi-2D perovskites
AU  - A. A. Gladkij
AU  - N. N. Rosanov
AU  - B. D. Fainberg
PY  - 2026
DA  - 2026/09/08
PB  - arXiv
DO  - 10.48550/arxiv.2609.08513
UR  - https://arxiv.org/abs/2609.08513
AB  - Recently, a soliton mechanism for room-temperature superfluorescence in thin perovskite films has been proposed, with a fundamental soliton predicted to remain stable under LO phonon--exciton interactions. At the same time, superlattice architectures offer a route to enhancing superfluorescence in perovskites. Motivated by recent observations of room-temperature superfluorescence in periodic superlattices of quasi-2D metal-halide perovskites, we extend the 2D nonlocal nonlinear Schrödinger equation describing Wannier exciton--LO phonon interactions to superlattice structures, obtaining a 3D nonlocal nonlinear Schrödinger equation. We show that interlayer tunnelling gives rise to breather dynamics corresponding to a stable fundamental soliton in mixed coordinate--momentum space, with the coordinate parallel to the layers and the momentum perpendicular to them. The breather dynamics originate from miniband formation, which induces a momentum-dependent phase modulation of the soliton. In the absence of interlayer tunnelling, the breather dynamics disappear and the soliton becomes stationary. These results establish a direct connection between interlayer tunnelling, miniband formation and soliton dynamics, suggesting that breather behavior can provide a signature of interlayer tunnelling in quasi-2D perovskite superlattices.
ER  -