Skip to content
DraconiticResearch
Search Sources API
201,818 studies31 sourcesUpdated just now
PreprintarXiv licencearXiv

Limitations of Debye-Waller lattice temperature extraction under electronic excitation

Abstract

Ultrafast diffraction is the cutting-edge technique to extract the atomic temperature at femtosecond timescales, and further related quantities - in particular, electron-phonon coupling strength at elevated electronic temperatures. The present work demonstrates limitations of such an analysis, emphasizing the importance of careful evaluation of the evolution of the Debye temperature. It is shown that, due to the sensitivity of the Debye-Waller analysis to this parameter, neglecting its changes under electronic excitation may lead to significant deviations of the atomic temperature extracted from its true values.

Related

  1. Nonequilibrium Electronic Response Modes Link Excitation Energy to Catalytic Reactivity
    Mengru Li, Hao Wang, Hui Yin
    ChemRxivPreprintCC BYAtomic, molecular & optical physicsChemRxiv
  2. Electronic-Structure Control of Nuclear Excitation by Electron Capture in Finite-Density 229Th
    Yang-Yang Xu, Jin-Tao Qi, Qiong Xiao +4
    arXivPreprintarXiv licenceFull textAtomic, molecular & optical physicsNuclear physicsarXiv
  3. Probing fluctuations in photon emission statistics of spin injected quantum dots with time dependent electronic excitation
    Chiran Wijesundara, Vincent Iglesias-Cardinale, Yuan Lu +3
    arXivPreprintCC0Full textCondensed matterQuantum physics & quantum informationarXiv
  4. Excitation of non-modal perturbations in hypersonic boundary layers by free stream forcing. Part III: effects of wall temperature and nose bluntness
    Lei Zhao, Mingze Sun, Qinyang Song +1
    arXivPreprintarXiv licenceFull textFluid dynamicsarXiv
  5. Extraction of different electronic contributions to transport properties of transition metals from first principles
    I. S. Galtsov, D. V. Minakov, P. R. Levashov
    arXivPreprintarXiv licenceFull textCondensed matterarXiv
BibTeX
@misc{medvedev2026limitations,
  title = {{Limitations of Debye-Waller lattice temperature extraction under electronic excitation}},
  author = {N. Medvedev and M. Kopecky and J. Chalupsky and L. Juha},
  howpublished = {arXiv},
  year = {2026},
  month = oct,
  doi = {10.48550/arxiv.2605.15140},
  eprint = {2605.15140},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2605.15140},
}
RIS
TY  - UNPB
TI  - Limitations of Debye-Waller lattice temperature extraction under electronic excitation
AU  - N. Medvedev
AU  - M. Kopecky
AU  - J. Chalupsky
AU  - L. Juha
PY  - 2026
DA  - 2026/10/23
PB  - arXiv
DO  - 10.48550/arxiv.2605.15140
UR  - https://arxiv.org/abs/2605.15140
AB  - Ultrafast diffraction is the cutting-edge technique to extract the atomic temperature at femtosecond timescales, and further related quantities - in particular, electron-phonon coupling strength at elevated electronic temperatures. The present work demonstrates limitations of such an analysis, emphasizing the importance of careful evaluation of the evolution of the Debye temperature. It is shown that, due to the sensitivity of the Debye-Waller analysis to this parameter, neglecting its changes under electronic excitation may lead to significant deviations of the atomic temperature extracted from its true values.
ER  -