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PreprintarXiv licencearXiv

Cathodoluminescence Wavefront Retrieval

Abstract

Free-electron-based nanoscopy enables the study of optical excitations in materials with deep-subwavelength spatial resolution, with cathodoluminescence (CL) being one of the most useful resulting signals. When combined with an optical collection system, CL measurements can access multidimensional information of light; yet the phase of the emitted optical fields has remained largely elusive. Here, we demonstrate a reference-free phase retrieval approach for far-field CL wavefronts using the Gerchberg-Saxton algorithm implemented with real-space and angular-space CL intensity data. Applying this approach to representative nanostructures, including a planar surface, nanosphere, plasmonic crystal, and nanowire, we reconstruct distinct phase distributions that reveal their underlying radiation mechanisms. This reference-free framework offers a robust and flexible route for retrieving the phase of electron-beam-excited optical fields without relying on a reference wave, making it readily extendable to a wide range of nanostructures.

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BibTeX
@misc{machfuudzoh2026cathodoluminescence,
  title = {{Cathodoluminescence Wavefront Retrieval}},
  author = {Izzah Machfuudzoh and Ryoichi Horisaki and Takumi Sannomiya},
  howpublished = {arXiv},
  year = {2026},
  month = oct,
  doi = {10.48550/arxiv.2605.21944},
  eprint = {2605.21944},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2605.21944},
}
RIS
TY  - UNPB
TI  - Cathodoluminescence Wavefront Retrieval
AU  - Izzah Machfuudzoh
AU  - Ryoichi Horisaki
AU  - Takumi Sannomiya
PY  - 2026
DA  - 2026/10/10
PB  - arXiv
DO  - 10.48550/arxiv.2605.21944
UR  - https://arxiv.org/abs/2605.21944
AB  - Free-electron-based nanoscopy enables the study of optical excitations in materials with deep-subwavelength spatial resolution, with cathodoluminescence (CL) being one of the most useful resulting signals. When combined with an optical collection system, CL measurements can access multidimensional information of light; yet the phase of the emitted optical fields has remained largely elusive. Here, we demonstrate a reference-free phase retrieval approach for far-field CL wavefronts using the Gerchberg-Saxton algorithm implemented with real-space and angular-space CL intensity data. Applying this approach to representative nanostructures, including a planar surface, nanosphere, plasmonic crystal, and nanowire, we reconstruct distinct phase distributions that reveal their underlying radiation mechanisms. This reference-free framework offers a robust and flexible route for retrieving the phase of electron-beam-excited optical fields without relying on a reference wave, making it readily extendable to a wide range of nanostructures.
ER  -