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Peer-reviewedCC BYAdvanced Materials

Robust Spin Splitting and Fermiology in the Layered Altermagnet CoNb4Se8

36 more authors
38 affiliations
  1. 1Fritz Haber Institut der Max Planck Gesellschaft Berlin Germany
  2. 2Institut für Physik und Astronomie Technische Universität Berlin Berlin Germany
  3. 3FHI - Fritz-Haber-Institut der Max-Planck-Gesellschaft (Faradayweg 4-6- D-14195 Berlin - Germany)
  4. 4Synchrotron SOLEIL Saint‐Aubin France
  5. 5SSOLEIL - Synchrotron SOLEIL (L'Orme des Merisiers Saint-Aubin - BP 48 91192 GIF-sur-YVETTE CEDEX - France)
  6. 6Centre de Nanosciences et de Nanotechnologies Université Paris‐Saclay, CNRS Paris France
  7. 7C2N - Centre de Nanosciences et de Nanotechnologies (10 Boulevard Thomas Gobert, 91120, Palaiseau - France)
  8. 8Université Paris-Saclay (Bâtiment Bréguet, 3 Rue Joliot Curie 2e ét, 91190 Gif-sur-Yvette - France)
  9. 9Diamond Light Source Ltd Harwell Science and Innovation Campus Didcot UK
  10. 10DIAMOND Light source (Diamond House, Harwell Science and Innovation Campus, Didcot, Oxfordshire OX11 0DE - United Kingdom)
  11. 11Université Paris‐Saclay Versailles France
  12. 12GEMAC - Groupe d'Etude de la Matière Condensée (URF de Sciences Bâtiment Fermat 45 avenue des Etats Unis 78035 Versailles - France)
  13. 13Department of Physics and Astronomy, Interdisciplinary Nanoscience Center Aarhus University Aarhus C Denmark
  14. 14IOM - CNR Istituto Officina dei Materiali (Laboratorio TASC Area Science Park - Basovizza Ed.MM, Strada Statale 14 Km 163,5 I-34149 Trieste - Italy)
  15. 15CNR‐Istituto Officina dei Materiali (IOM) Unità di Trieste Basovizza (TS) Italy
  16. 16Dipartimento di Fisica Università degli Studi di Trieste Trieste Italy
  17. 17Elettra ‐ Sincrotrone Trieste S.C.p.A. Trieste Italy
  18. 18CNR-SPIN and Department of Physics “E. Pancini (Piazzale V. Tecchio 80, I-80125 Naples - Italy)
  19. 19CNR‐SPIN Universitá di Salerno Fisciano (SA) Italy
  20. 20NBI - Niels Bohr Institute [Copenhagen] (Blegdamsvej 17, DK-2100 Copenhagen - Denmark)
  21. 21Niels Bohr Institute University of Copenhagen Copenhagen Denmark
  22. 22Monash University [Clayton] (Clayton, VIC 3800, Australia - Australia)
  23. 23School of Physics and Astronomy Monash University Victoria Australia
  24. 24Department of Physics Boston College Chestnut Hill Massachusetts USA
  25. 25ETH Zürich Zürich Switzerland
  26. 26Institute for Theoretical Physics and Astrophysics University of Würzburg Würzburg Germany
  27. 27CNR‐SPIN Complesso di Monte S. Angelo Napoli Italy
  28. 28Physics Department University of Napoli “Federico II” Napoli Italy
  29. 29Nanoscience Center, Niels Bohr Institute University of Copenhagen Copenhagen Denmark
  30. 30European Spallation Source ERIC ‐ Data Management and Software Center Kgs. Lyngby Denmark
  31. 31Faculty of Physics and Applied Computer Science AGH University of Krakow Krakow Poland
  32. 32Center for Artificial Low‐Dimensional Electronic Systems Institute for Basic Science Namgu Pohang Republic of Korea
  33. 33Department of Physics Pohang University of Science and Technology Pohang‐si Gyeongsangbuk‐do Republic of Korea
  34. 34Univ. Grenoble Alpes, CEA, CNRS, IRIG‐SPINTEC Grenoble France
  35. 35Electricity and Electronics and Semiconductor Applications Ulsan College Ulsan Republic of Korea
  36. 36Department of Physics University of Trento Povo Italy
  37. 37CNR‐Istituto di Struttura della Materia (CNR‐ISM) Trieste Italy
  38. 38Department of Physics and Astronomy ‘Galileo Galilei' University of Padova Padova Italy

Abstract

Altermagnetism defies conventional classifications of collinear magnetic phases, combining compensated magnetization with momentum‐dependent, nonrelativistic spin splitting. While altermagnetic band splitting has been established in three‐dimensional compounds such as MnTe and CrSb, layered altermagnets remain far less explored spectroscopically. Here, combining termination‐resolved micro‐ARPES, fine photon‐energy mapping, spin‐ARPES, and density functional theory, we map the three‐dimensional fermiology of the layered g ‐wave altermagnet , obtained by ordered Co intercalation of 2H‐. We resolve the spin–split branches of the altermagnetic pairs directly in the raw photoemission spectra and, with spin‐ARPES at these experimentally identified momenta, show the reversal of the spin polarization at opposite momenta and between two regions of the sample, consistent with opposite time‐reversal domains, and its absence along the symmetry‐protected nodal –K direction. We further report a weak low‐temperature anomaly near T 0 ≈ 50–60 K, detected by magnetometry, temperature‐dependent micro‐ARPES, and ultrafast reflectivity, whose microscopic origin remains open. These results provide a momentum‐resolved benchmark of the electronic structure of a layered altermagnet.

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BibTeX
@article{vita2026robust,
  title = {{Robust Spin Splitting and Fermiology in the Layered Altermagnet CoNb4Se8}},
  author = {Alessandro De Vita and Chiara Bigi and Davide Romanin and Matthew D. Watson and Vincent Polewczyk and Marta Zonno and F. Bertran and Pietro Maria Forcella and My Bang Petersen and Federico Motti and Giovanni Vinai and Manuel Tuniz and Federico Cilento and Mario Cuoco and Brian M. Andersen and Andreas Kreisel and Luciano Jacopo D’Onofrio and Oliver J. Clark and Mark T. Edmonds and Christopher Candelora and Muxian Xu and Siyu Cheng and Alexander LaFleur and Tommaso Antonelli and Giorgio Sangiovanni and Lorenzo Del Re and I. Vobornik and Jun Fujii and F. Miletto Granozio and A. Sambri and Emiliano Di Gennaro and H. Jacobsen and H. Jacobsen and Iulia Cojocariu and Marcin Szpytma and Andrea Locatelli and Tevfik Onur Menteş and Won Seop Song and Jun Sung Kim and Matthieu Jamet and Jean‐François Jacquot and P. Orgiani and Ralph Ernstorfer and Ilija Zeljkovic and Y. T. Hwang and Jill A. Miwa and Jill A. Miwa and Federico Mazzola},
  journal = {Advanced Materials},
  year = {2026},
  month = oct,
  doi = {10.1002/adma.75367},
  url = {https://doi.org/10.1002/adma.75367},
  note = {CC BY},
}
RIS
TY  - JOUR
TI  - Robust Spin Splitting and Fermiology in the Layered Altermagnet CoNb4Se8
AU  - Alessandro De Vita
AU  - Chiara Bigi
AU  - Davide Romanin
AU  - Matthew D. Watson
AU  - Vincent Polewczyk
AU  - Marta Zonno
AU  - F. Bertran
AU  - Pietro Maria Forcella
AU  - My Bang Petersen
AU  - Federico Motti
AU  - Giovanni Vinai
AU  - Manuel Tuniz
AU  - Federico Cilento
AU  - Mario Cuoco
AU  - Brian M. Andersen
AU  - Andreas Kreisel
AU  - Luciano Jacopo D’Onofrio
AU  - Oliver J. Clark
AU  - Mark T. Edmonds
AU  - Christopher Candelora
AU  - Muxian Xu
AU  - Siyu Cheng
AU  - Alexander LaFleur
AU  - Tommaso Antonelli
AU  - Giorgio Sangiovanni
AU  - Lorenzo Del Re
AU  - I. Vobornik
AU  - Jun Fujii
AU  - F. Miletto Granozio
AU  - A. Sambri
AU  - Emiliano Di Gennaro
AU  - H. Jacobsen
AU  - H. Jacobsen
AU  - Iulia Cojocariu
AU  - Marcin Szpytma
AU  - Andrea Locatelli
AU  - Tevfik Onur Menteş
AU  - Won Seop Song
AU  - Jun Sung Kim
AU  - Matthieu Jamet
AU  - Jean‐François Jacquot
AU  - P. Orgiani
AU  - Ralph Ernstorfer
AU  - Ilija Zeljkovic
AU  - Y. T. Hwang
AU  - Jill A. Miwa
AU  - Jill A. Miwa
AU  - Federico Mazzola
PY  - 2026
DA  - 2026/10/18
JO  - Advanced Materials
DO  - 10.1002/adma.75367
UR  - https://doi.org/10.1002/adma.75367
AB  - Altermagnetism defies conventional classifications of collinear magnetic phases, combining compensated magnetization with momentum‐dependent, nonrelativistic spin splitting. While altermagnetic band splitting has been established in three‐dimensional compounds such as MnTe and CrSb, layered altermagnets remain far less explored spectroscopically. Here, combining termination‐resolved micro‐ARPES, fine photon‐energy mapping, spin‐ARPES, and density functional theory, we map the three‐dimensional fermiology of the layered g ‐wave altermagnet , obtained by ordered Co intercalation of 2H‐. We resolve the spin–split branches of the altermagnetic pairs directly in the raw photoemission spectra and, with spin‐ARPES at these experimentally identified momenta, show the reversal of the spin polarization at opposite momenta and between two regions of the sample, consistent with opposite time‐reversal domains, and its absence along the symmetry‐protected nodal –K direction. We further report a weak low‐temperature anomaly near T 0 ≈ 50–60 K, detected by magnetometry, temperature‐dependent micro‐ARPES, and ultrafast reflectivity, whose microscopic origin remains open. These results provide a momentum‐resolved benchmark of the electronic structure of a layered altermagnet.
SN  - 0935-9648
SN  - 1521-4095
ER  -