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PreprintCC BY 4.0arXiv

Interface engineering of spin triplet Cooper pairs for spin-valve implementation

Abstract

Spin singlet Cooper pairs can be converted into equal-spin triplet pairs at a superconductor/heavy-metal interface under suitable conditions. Under current carrying conditions, these triplet correlations can give rise to a non equilibrium spin moment in the heavy metal through the predicted supercurrent spin-Hall effect. Here we demonstrate that this current induced triplet spin moment, in conjunction with the magnetic moment of a ferromagnetic layer, can enable a magnetic spin-valve response in Nb/Pt/Ni/Pt/Nb vertical nano-devices. The magnitude of this spin-valve effect depends on the efficiency of singlet-triplet Cooper pair conversion at the Nb/Pt interface. In order to facilitate efficient triplet generation, we deliberately introduced interfacial roughness to introduce finite Rashba spin-orbit coupling at the Nb/Pt interface and an out-of-plane component of magnetic moment at the Ni interface. In contrast, no discernible spin-valve response was observed in devices with smooth interfaces within measurement resolutions. Since the magnetic moment of the Ni layer and the current-induced triplet spin moment in the Pt layer are independently switchable using a magnetic field and bias current, respectively, the spin valve can be controlled via either parameters. These results demonstrates a novel approach to directly utilizing the spin polarized triplet Copper pairs in superconducting spintronic applications.

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BibTeX
@misc{nayak2026interface,
  title = {{Interface engineering of spin triplet Cooper pairs for spin-valve implementation}},
  author = {Debashree Nayak and Abhisek Sahoo and Pratap Kumar Sahoo and Kartik Senapati},
  howpublished = {arXiv},
  year = {2026},
  month = sep,
  doi = {10.48550/arxiv.2609.24803},
  eprint = {2609.24803},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2609.24803},
  note = {CC BY 4.0},
}
RIS
TY  - UNPB
TI  - Interface engineering of spin triplet Cooper pairs for spin-valve implementation
AU  - Debashree Nayak
AU  - Abhisek Sahoo
AU  - Pratap Kumar Sahoo
AU  - Kartik Senapati
PY  - 2026
DA  - 2026/09/26
PB  - arXiv
DO  - 10.48550/arxiv.2609.24803
UR  - https://arxiv.org/abs/2609.24803
AB  - Spin singlet Cooper pairs can be converted into equal-spin triplet pairs at a superconductor/heavy-metal interface under suitable conditions. Under current carrying conditions, these triplet correlations can give rise to a non equilibrium spin moment in the heavy metal through the predicted supercurrent spin-Hall effect. Here we demonstrate that this current induced triplet spin moment, in conjunction with the magnetic moment of a ferromagnetic layer, can enable a magnetic spin-valve response in Nb/Pt/Ni/Pt/Nb vertical nano-devices. The magnitude of this spin-valve effect depends on the efficiency of singlet-triplet Cooper pair conversion at the Nb/Pt interface. In order to facilitate efficient triplet generation, we deliberately introduced interfacial roughness to introduce finite Rashba spin-orbit coupling at the Nb/Pt interface and an out-of-plane component of magnetic moment at the Ni interface. In contrast, no discernible spin-valve response was observed in devices with smooth interfaces within measurement resolutions. Since the magnetic moment of the Ni layer and the current-induced triplet spin moment in the Pt layer are independently switchable using a magnetic field and bias current, respectively, the spin valve can be controlled via either parameters. These results demonstrates a novel approach to directly utilizing the spin polarized triplet Copper pairs in superconducting spintronic applications.
ER  -