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Peer-reviewedCC BY 4.0PLOS One

Cradle-to-gate life cycle assessment of sisal/PLA biocomposite: Uncovering the dominance of transport and burden-shifting trade-offs in sustainable material design

  1. 1School of Materials, Energy, Water and Environmental Science (MEWES), The Nelson Mandela African Institution of Science and Technology (NM-AIST), Arusha, Tanzania
  2. 2Department of Business Management, The Mbeya University of Science and Technology (MUST), Mbeya, Tanzania
  3. 3School of Business Studies and Humanities (BuSH), The Nelson Mandela African Institution of Science and Technology (NM-AIST), Arusha, Tanzania

Abstract

Natural fibre-reinforced biocomposites are increasingly recognised as promising alternatives for reducing the high carbon footprint of the construction sector; however, the environmental implications of transcontinental supply chains remain insufficiently understood. This study presents a cradle-to-gate life cycle assessment of a sisal yarn-reinforced polylactic acid biocomposite plate manufactured in Denmark using sisal fibres cultivated and spun in Tanzania. Environmental impacts were assessed for a performance-based functional unit using the ReCiPe 2016 Midpoint (H) method, normalising values through a structural bending stiffness index to enable benchmarking against conventional window frame materials. Under baseline pilot-scale conditions, the biocomposite exhibited a global warming potential of 17.52 kg of carbon dioxide equivalent, with intercontinental air freight accounting for 62.53% of total emissions. Scenario optimisation involving ocean freight, 100% wind energy, and a 60:40 polylactic acid-to-sisal ratio reduced the global warming potential to 9.82 kg of carbon dioxide equivalent, a 43.97% reduction. When normalised for structural performance, the optimised biocomposite demonstrated a lower global warming potential than conventional polyvinyl chloride and aluminium window frame materials. Nevertheless, these improvements resulted in significant shifts in environmental burdens, with human non-carcinogenic toxicity increasing by 125.91% and freshwater ecotoxicity by 322.88%, primarily due to heavy fuel oil combustion during marine transport and the use of synthetic phosphate fertiliser in sisal cultivation. The findings indicate that although transcontinental sisal/polylactic acid biocomposites can offer competitive structural and climate performance, their long-term sustainability depends on holistic multi-indicator assessments and the adoption of cleaner logistics and sustainable agricultural practices to avoid transferring environmental burdens across impact categories.

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BibTeX
@article{kahigi2026cradletogate,
  title = {{Cradle-to-gate life cycle assessment of sisal/PLA biocomposite: Uncovering the dominance of transport and burden-shifting trade-offs in sustainable material design}},
  author = {Nickson Severian Kahigi and Revocatus Machunda and Josephine Joseph Mkunda and Mwema Felix Mwema},
  journal = {PLOS One},
  year = {2026},
  month = sep,
  doi = {10.1371/journal.pone.0349715},
  url = {https://doi.org/10.1371/journal.pone.0349715},
  note = {CC BY 4.0},
}
RIS
TY  - JOUR
TI  - Cradle-to-gate life cycle assessment of sisal/PLA biocomposite: Uncovering the dominance of transport and burden-shifting trade-offs in sustainable material design
AU  - Nickson Severian Kahigi
AU  - Revocatus Machunda
AU  - Josephine Joseph Mkunda
AU  - Mwema Felix Mwema
PY  - 2026
DA  - 2026/09/23
JO  - PLOS One
DO  - 10.1371/journal.pone.0349715
UR  - https://doi.org/10.1371/journal.pone.0349715
AB  - Natural fibre-reinforced biocomposites are increasingly recognised as promising alternatives for reducing the high carbon footprint of the construction sector; however, the environmental implications of transcontinental supply chains remain insufficiently understood. This study presents a cradle-to-gate life cycle assessment of a sisal yarn-reinforced polylactic acid biocomposite plate manufactured in Denmark using sisal fibres cultivated and spun in Tanzania. Environmental impacts were assessed for a performance-based functional unit using the ReCiPe 2016 Midpoint (H) method, normalising values through a structural bending stiffness index to enable benchmarking against conventional window frame materials. Under baseline pilot-scale conditions, the biocomposite exhibited a global warming potential of 17.52 kg of carbon dioxide equivalent, with intercontinental air freight accounting for 62.53% of total emissions. Scenario optimisation involving ocean freight, 100% wind energy, and a 60:40 polylactic acid-to-sisal ratio reduced the global warming potential to 9.82 kg of carbon dioxide equivalent, a 43.97% reduction. When normalised for structural performance, the optimised biocomposite demonstrated a lower global warming potential than conventional polyvinyl chloride and aluminium window frame materials. Nevertheless, these improvements resulted in significant shifts in environmental burdens, with human non-carcinogenic toxicity increasing by 125.91% and freshwater ecotoxicity by 322.88%, primarily due to heavy fuel oil combustion during marine transport and the use of synthetic phosphate fertiliser in sisal cultivation. The findings indicate that although transcontinental sisal/polylactic acid biocomposites can offer competitive structural and climate performance, their long-term sustainability depends on holistic multi-indicator assessments and the adoption of cleaner logistics and sustainable agricultural practices to avoid transferring environmental burdens across impact categories.
SN  - 1932-6203
ER  -