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PreprintarXiv licencearXiv

Hall-Density Collapse as Direct Evidence for Percolative Conduction Onset in Monolayer MoS2 Transistors

Abstract

The origin of the apparent metal-insulator transition in two-dimensional electron systems remains debated. Using temperature-dependent transport and Hall measurements on industry-relevant MoS2 monolayer FETs with amorphous HfO2 dielectrics, we establish classical percolation as the underlying mechanism. We report two complementary signatures of disorder-driven conduction onset: a temperature-independent Hall-density collapse as a function of absolute gate voltage and a vanishing activation energy at a characteristic carrier density nc, identified as the percolation threshold. These findings identify dielectric-interface disorder, rather than channel quality alone, as the key parameter governing device turn-on. The extracted activation barriers reach values substantially exceeding room-temperature thermal energies, indicating that disorder-driven conduction onset remains relevant well beyond cryogenic transport.

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BibTeX
@misc{upadya2026halldensity,
  title = {{Hall-Density Collapse as Direct Evidence for Percolative Conduction Onset in Monolayer MoS$_2$ Transistors}},
  author = {R. V. Upadya and M. Introna and X. Wu and C. J. L. de la Rosa and K. Banerjee and D. Lin and K. De Greve},
  howpublished = {arXiv},
  year = {2026},
  month = nov,
  doi = {10.48550/arxiv.2611.06815},
  eprint = {2611.06815},
  archivePrefix = {arXiv},
  url = {https://arxiv.org/abs/2611.06815},
}
RIS
TY  - UNPB
TI  - Hall-Density Collapse as Direct Evidence for Percolative Conduction Onset in Monolayer MoS_2 Transistors
AU  - R. V. Upadya
AU  - M. Introna
AU  - X. Wu
AU  - C. J. L. de la Rosa
AU  - K. Banerjee
AU  - D. Lin
AU  - K. De Greve
PY  - 2026
DA  - 2026/11/04
PB  - arXiv
DO  - 10.48550/arxiv.2611.06815
UR  - https://arxiv.org/abs/2611.06815
AB  - The origin of the apparent metal-insulator transition in two-dimensional electron systems remains debated. Using temperature-dependent transport and Hall measurements on industry-relevant MoS_2 monolayer FETs with amorphous HfO_2 dielectrics, we establish classical percolation as the underlying mechanism. We report two complementary signatures of disorder-driven conduction onset: a temperature-independent Hall-density collapse as a function of absolute gate voltage and a vanishing activation energy at a characteristic carrier density n_c, identified as the percolation threshold. These findings identify dielectric-interface disorder, rather than channel quality alone, as the key parameter governing device turn-on. The extracted activation barriers reach values substantially exceeding room-temperature thermal energies, indicating that disorder-driven conduction onset remains relevant well beyond cryogenic transport.
ER  -